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A<sc>bstract</sc> The first FASER search for a light, long-lived particle decaying into a pair of photons is reported. The search uses LHC proton-proton collision data at$$ \sqrt{s} $$ $\sqrt{s}$= 13.6 TeV collected in 2022 and 2023, corresponding to an integrated luminosity of 57.7 fb⁻¹. A model with axion-like particles (ALPs) dominantly coupled to weak gauge bosons is the primary target. Signal events are characterised by high-energy deposits in the electromagnetic calorimeter and no signal in the veto scintillators. One event is observed, compared to a background expectation of 0.44 ± 0.39 events, which is entirely dominated by neutrino interactions. World-leading constraints on ALPs are obtained for masses up to 300 MeV and couplings to the Standard Model W gauge boson,g_aWW, around 10⁻⁴GeV⁻¹, testing a previously unexplored region of parameter space. Other new particle models that lead to the same experimental signature, including ALPs coupled to gluons or photons, U(1)_Bgauge bosons, up-philic scalars, and a Type-I two-Higgs doublet model, are also considered for interpretation, and new constraints on previously viable parameter space are presented in this paper.